Sains Malaysiana 37(4):  401-404 (2008)

 

Assessment of Neutron Flux Gradients in Irradiation Channels at the

TRIGA Reactor by Au-Cr-Mo Monitor Set Based on k0-INAA

(Penilaian Tentang Kecerunan Fluks Neutron Dalam Saluran Penyinaran di Reaktor

TRIGA Dengan Set Pemonitor Au-Cr-Mo Berdasarkan ko-APNI)

 

Khoo Kok Siong & Ti Kien Leong

Nuclear Science Programme

School of Applied Physics, Faculty of Science and Technology

Universiti Kebangsaan Malaysia, 43600 Bangi, Selangor, Malaysia

 

 

Sukiman Sarmani & Amran Majid

Chemistry Programme, School of Chemical Sciences & Food Technology

Universiti Kebangsaan Malaysia, 43600 Bangi, Selangor, Malaysia

 

Received:  4 January 2008 / Accepted:  4 April 2008

 

ABSTRACT

A gradient of neutron flux distribution in an irradiation channel in research reactor is considered to have effect on the k0-instrumental neutron activation analysis (k0-INAA) measurement. A study has been carried out to determine: (1) the variation of the thermal to epithermal neutron flux ratio (f); (2) the epithermal neutron flux shape factor (α), and (3) the neutron flux in an irradiation container at four selected irradiation channels, use being made of an Au-Cr-Mo monitor set. In this work, f was found to range from 15.5 – 16.3, while α was found to range from 1.52 x 10-2 – 5.58 x 10-2. Additionally, within the selected irradiation channels the variation in calculated thermal neutron flux within one irradiation container was found to vary from 11.8% - 26.7%. The results of analysis have provided a determination of variation in the neutron parameters, f and α, and neutron flux between the irradiation channels and within the irradiation container.

 

Keywords: k0-INAA; neutron flux distribution; neutron parameters

 

 

ABSTRAK

 

Kecerunan taburan fluks neutron pada saluran penyinaran dalam reaktor penyelidikan boleh memberikan kesan kepada pengukuran analisis pengaktifan neutron instrumentasi k0 (k0-APNI). Satu kajian telah dilakukan untuk menentukan: (1) variasi nisbah fluks neutron terma kepada fluks neutron epiterma (f); (2) faktor pembentukan fluks neutron epiterma (α), dan (3) fluks neutron dalam satu bekas penyinaran pada empat saluran penyinaran terpilih dengan menggunakan set pemantau Au-Cr-Mo. Dalam kerja ini, f adalah dalam julat 15.5 – 16.3 dan α menunjukkan julat di antara 1.52 x 10-2 – 5.58 x 10-2. Tambahan, variasi fluks neutron terma yang dikira dalam satu bekas penyinaran mempunyai perbezaan dari 11.8% - 26.7% pada saluran penyinaran terpilih. Keputusan analisis membuktikan terdapat variasi dalam parameter neutron, f dan α, serta fluks neutron di antara saluran penyinaran dan dalam bekas penyinaran.

 

Kata kunci: k0-APNI; taburan fluks neutron ; parameter neutron        

 

REFERENCES/RUJUKAN

Abugassa, I. 1999. A study of instrumental neutron activation analysis based on k0-standardization method developed for environmental materials. Ph.D Thesis. Bangi: Universiti Kebangsaan Malaysia.

Ammerlaan, M.J.J., Bacchi, M.A., Bode, P. & De Nadai Fernandes, E.A. 2004. Validation of a new kit for easy thermal and epithermal neutron flux monitoring. Transactions of the American Nuclear Society 91: 872-873.

Bode, P., Blaauw, M. & Obrusnik, I. 1992. Variation of neutron flux and related parameters in an irradiation container, in use with k0-based neutron activation analysis. Journal of Radioanalytical and Nuclear Chemistry 157(2): 301-312.

Canberra. 1993. Canberra model S342 SAMPO 90 V3.20 user’s manual. Meriden: Canberra Industries Inc.

Crow, M.L., Jeng, U., Nunes, A.C., Malik, S.S., Lin, D., Bai, S., Tehan, T., Jacob, N., Johnson, D.G., Simoneau, W.A. & Dimeglio, A.F. 1995. Thermal neutron measurements of the Rhode Island Nuclear Science Center reactor after conversion to a compact low enriched uranium core. Nuclear Instruments and Methods in Physics Research A 365: 433 – 445.

De Corte, F. 1987. The k0-standardization method: A move to the optimization of NAA. Agrege Thesis. Belgium: University of Gent.

De Corte, F. & Simonits, A. 1994. Vade mecum for k0-users. Geleen (NL): DSM Research.

Hala, J. 1992. Nuclear chemistry. West Sussex: Ellis Horwood Ltd.

Jacimovic, R., Stibilj, V., Benedik, L. & Smodis, B. 2003. Characterization of the neutron flux gradients in typical irradiation channels of a TRIGA Mark II reactor. Journal of Radioanalytical and Nuclear Chemistry 257(3): 545-549.

Khoo, K.S., Sarmani, S.B. & Abugassa, I.O. 2007. Determination of thermal to epithermal neutron flux ratio (f), epithermal neutron shape factor (a) and comparator factor (Fc) in the TRIGA Mark II reactor. Journal of Radioanalytical and Nuclear Chemistry 271:  419 - 424.

Lin, X, Alber, D. & Henkelmann, R. 2003. Calibration of the irradiation channel DBVK at BER-II reactor and feasibility of applying the k0-method at this device. Journal of Radioanalytical and Nuclear Chemistry 257:  531-538.

Simonits, A., De Corte, F. & Hoste, J. 1975. Single–comparator methods in reactor neutron activation analysis. Journal of Radioanalytical and Chemistry 24: 31-46.

Wee, B.S., Ho, M.D., Wood, A.K., Salim, N.A.A. & Elias, M.S. 2006. Testing the applicability of the k0-NAA method at the MINT’s TRIGA MARK II reactor. Nuclear Instruments & Methods in Physics Research A 564: 716-720.

 

 

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